sputneek: This way-too-cool bike-surfshop cum café tucked in a Harajuku lane serves really good coffee. Sandwiches are hearty meals with fries and salad. Really nice place to just 'zone out' from the crowd.
Arjan Timmermans: Fantastic modern-art museum. Large building that houses special exhibits and a rotating selection of its collection. If you want to get a taste of avant-garde Tokyo, this is the place for you.